【507】Circular Dichroism and Orbital Angular Momentum in chiral Weyl semimetals PdGa/PtGa

5 Sept 2023, 15:45
15m
Room 115

Room 115

Talk New prospects in ARPES for quantum materials New prospects in ARPES for quantum materials

Speaker

Yun Yen (Paul Scherrer Institute / EPFL)

Description

In this work, we show that circular dichroism angle resolved photoemission spectroscopy (CD-ARPES) can map topology in chiral Weyl semimetals PdGa/PtGa, where multifold nodes host large Chern number[1,2]. We successfully simulate the CD intensity using our in-house code dynamics-w90[3]. The correspondence between local OAM and dipole matrix elements depends on orbital characters and experimental geometry. Pd/Pt local OAM can be measured by CD, where d orbital contribution is dominated by m=∓2 complex orbitals. Although the total CD signal consists of interatomic interference terms, they still exhibit radial structure. We conclude that one can see the reminiscence of radial OAM structure, which comes from the topological nature of the Weyl nodes.

Theoretical Work Theory

Authors

Dr Iñigo Robredo (Max Planck Institute for Chemical Physics of Solids) Dr Jonas A. Krieger (Max Planck Institute of Microstructure Physics) Dr Maia G. Vergniory (Donostia International Physics Center) Dr MengYu Yao (Max Planck Institute for Chemical Physics of Solids) Prof. Michael Schüler (Paul Scherrer Institute / Department of Physics, University of Fribourg) Dr Niels B. M. Schröter (Max Planck Institute of Microstructure Physics) Dr Qun Yang (Weizmann Institute of Science) Yun Yen (Paul Scherrer Institute / EPFL)

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