【224】Optimized Infrared Reflection Absorption Spectroscopy for Metal Oxides: Overcoming Challenges of Low Reflectivity and Sub-Monolayer Coverage

7 Sept 2023, 17:45
15m
Room 114

Room 114

Talk Surfaces, Interfaces and Thin Films Surfaces, Interfaces and Thin Films

Speaker

Jiri Pavelec (Vienna University of Technology)

Description

This study presents a new Infrared Reflection Absorption Spectroscopy (IRAS) setup for investigating adsorption on "single-atom" catalysts, addressing the challenges of low reflectivity from oxide supports and sub-monolayer coverage of adsorbates. The setup features improvements such as a high numerical aperture, optimized optical path, controlled incidence angle range, and high mechanical stability. Utilizing adjustable aperture plates, the minimum and maximum incidence angles can be varied to optimize the signal for each sample. This new setup successfully demonstrated enhanced signal-to-noise ratio in D2O and CO absorbance measurements on a rutile TiO2(110) surface, agreeing with established literature, with significantly reduced measurement time.

Authors

Jiri Pavelec (Vienna University of Technology) David Rath (Vienna University of Technology) Michael Schmid (Vienna University of Technology) Ulrike Diebold (Vienna University of Technology) Gareth Parkinson (Vienna University of Technology)

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