【116】Mixed singlet and triplet two-hole states in Bi2Sr2CaCu2O8+δ unveiled by cluster modeling of the d-d excitations observed by Resonant Inelastic X-Ray Scattering

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15m
Talk Condensed Matter Physics (KOND) Condensed Matter Physics (KOND)

Speaker

Wenliang Zhang (Swiss Light Source, Paul Scherrer Institut)

Description

We studied the d-d excitations in Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ by Cu L$_3$-edge Resonant Inelastic X-ray Scattering with azimuthal rotation of the polarizations in the sample space, and analyzed the experimental response with a single cluster model. Utilizing group theory classification to incorporate two-hole Coulomb interactions via a Green's function approach, the calculations suggest that the d-d excitations can be described by a two-hole ground state composed of a Hund’s triplet mixed with a Zhang-Rice singlet state in all the studied doping regions. Our results highlight the existence of the spin-triplet two-hole state for doped cuprates, and that Hund’s triplet physics could play a role in the optimally doped and over-doped regions.

Authors

Mr Meiyu He (State Key Laboratory of Optoelectronic Materials and Technologies, School of Physics, Sun Yat-Sen University) Wenliang Zhang (Swiss Light Source, Paul Scherrer Institut) Prof. Dao-Xin Yao (State Key Laboratory of Optoelectronic Materials and Technologies, School of Physics, Sun Yat-Sen University) Prof. Trinanjan Datta (The Department of Physics and Biophysics, Augusta University) Thorsten Schmitt (Swiss Light Source, Paul Scherrer Institute)

Co-authors

Yi Tseng (Paul Scherrer Institut) Teguh Citra Asmara (Paul Scherrer Institute) Eugenio Paris (PSI - Paul Scherrer Institut) Dr Vladimir N. Strocov (Swiss Light Source, Paul Scherrer Institut) Enrico Giannini (University of Geneva)

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