9–13 Sept 2024
ETH Zürich
Europe/Zurich timezone

【101】Coupled magnetism and ferroelectricity in magnetic high entropy oxide

10 Sept 2024, 14:00
15m
ETZ E 7

ETZ E 7

Talk Condensed Matter Physics (KOND) Condensed Matter Physics (KOND)

Speaker

Roxana Capu (West University of Timisoara, Romania)

Description

Using low energy Muons spin rotation spectroscopy, measurement of dc/ac magnetic susceptibility and measurement of capacitance, we show that epitaxially grown Nd-based perovskite high entropy oxides exhibit significant ferromagnetism, spin-glass behaviour, high dielectric constant at RT and a temperature-dependent ferroelectric hysteresis that are intricately coupled to each other. X-ray absorption spectroscopy at 3d transition metal edges indicates a mixed valence state - possibly originating from the off-centring of the B-sites- that helps to explain these properties. These materials could be useful for exploiting magnetostriction and other related properties leading to next-generation sensors.

Authors

Roxana Capu (West University of Timisoara, Romania) Subhrangsu Sarkar

Co-authors

Ryan Thompson (University of Fribourg) Dr C. Willem Rischau (University of Geneva, Switzerland) Dr Marli R. Cantarino (ESRF, Grenoble, France) Dr Stefan Schuppler (Institute for Quantum Materials and Technologies(IQMT), Karlsruhe Institute of Technology(KIT), Germany) Dr Sergey Budko (Ames Laboratory, U.S.A) Stefano Gariglio (Université de Genève) Zaher Salman Prof. Yurii Pashkevich (University of Fribourg, Department of Physics and Fribourg Center for Nanomaterials, University of Fribourg, Fribourg CH-1700,Switzerland; O. Galkin Donetsk Institute for Physics and Engineering NAS of Ukraine, Ukraine) Christian Bernhard (Fribourg University)

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