9–13 Sept 2024
ETH Zürich
Europe/Zurich timezone

【514】Exploring Low-Energy Excitations and Magnetic Dichroism in Resonant Inelastic X-ray Scattering of the Ferromagnetic van der Waals Material VI$_{3}$

11 Sept 2024, 18:15
15m
ETF E 1

ETF E 1

Talk Electron and photon spectroscopies of quantum materials Electron and photon spectroscopies of quantum materials

Speaker

Yuan Wei

Description

The ferromagnetic van der Waals Material VI$_{3}$ is proposed as a Mott insulator with S = 1 state. A distinct symmetry breaking indicative of the FM transition is observed in the Raman spectra of monolayer samples. This study investigates low-energy excitations in VI$_{3}$ using high-resolution resonant inelastic X-ray scattering (RIXS). We identify the spin wave, revealing insights into the spin dynamics and exchange interactions, and unveil an orbital redistribution through the RIXS magnetic circular dichroism (MCD), underscoring the significance of orbital degrees of freedom in the magnetism. Our findings illustrate the sensitivity of RIXS-MCD in probing ferromagnetic van der Waals materials.

Primary author

Yuan Wei

Co-authors

Wenliang Zhang (Paul Scherrer Institut) Mr Zhen Tao (Paul Scherrer Institut) Teguh Citra Asmara (Paul Scherrer Institut) Tianlun Yu (Paul Scherrer Institut) Dr Mirian Garcia-Fernandez (Diamond Light Source, UK) Dr Cedomir Petrovic (Brookhaven National Laboratory, USA) Ke-Jin Zhou (Diamond Light Source, UK) Thorsten Schmitt (Paul Scherrer Institut)

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