9–13 Sept 2024
ETH Zürich
Europe/Zurich timezone

【515】Spin-orbital correlations in the van der Waals magnet CrPS4 revealed by resonant inelastic X-ray scattering

11 Sept 2024, 18:30
15m
ETF E 1

ETF E 1

Talk Electron and photon spectroscopies of quantum materials Electron and photon spectroscopies of quantum materials

Speaker

Zhijia Zhang

Description

Exfoliable magnetic van der Waals (vdW) materials have enabled the study of magnetism at the true two-dimensional limit. Bulk CrPS4 is an A-type vdW antiferromagnet with strong correlation between the electronic, orbital, structural properties and the magnetic state. I will present our temperature-dependent resonant inelastic X-ray scattering (RIXS) data: the linear-dichroic RIXS intensity of one of the orbital excitations shows an order-parameter-like temperature dependence around the Néel temperature (38 K). I will discuss this temperature-dependent orbital asymmetry in relation to our multiplet simulations, and how the RIXS dichroism of this orbital excitation will allow access to the magnetic state in future RIXS investigations of exfoliated flakes of this topical material.

Primary authors

Zhijia Zhang Yuan Wei carlos galdino (Paul Scherrer Institute) Wenliang Zhang Tianlun Yu Dr Thorsten Schmitt (Paul Scherrer Institut)

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