9–13 Sept 2024
ETH Zürich
Europe/Zurich timezone

【802】Imaging Ultrafast Electronic Domain Fluctuations in a Nonequilibrium X-Ray Speckle Visibility Experiment

13 Sept 2024, 13:45
15m
ETF E 1

ETF E 1

Talk Photon Science Photon Science

Speaker

Nelson Nientsu Hua (Paul Scherrer Institut)

Description

We employed a novel coherent X-ray technique that uses a split-and-delay line in a pump-double-probe experimental scheme to measure ultrafast domain fluctuations for the first time at an X-ray free electron laser. By accessing the speckle pattern of a resonant charge order peak in Fe$_{3}$O$_{4}$, we imaged electronic domain fluctuations with sub-picosecond temporal resolution. Here we also demonstrate how a standard time-resolved x-ray diffraction experiment in a pump-probe setup complements the coherent X-ray experiment by revealing how the average and local domain structures evolve in Fe$_{3}$O$_{4}$, offering a unique perspective on the ultrafast dynamics of the lattice structure and
electronic heterogeneities.

Authors

Aidan McConnell (Paul Scherrer Institut) Boyan Stoychev (University of California San Diego) Diling Zhu (SLAC National Accelerator Laboratory) Eric E. Fullerton (University of California San Diego) Erik Lamb (University of California San Diego) Henrik Lemke (Paul Scherrer Institut) Mathias Sander (Paul Scherrer Institut) Maël Clémence (Paul Scherrer Institut) Meera Madhavi (University of California Davis) Nanna Zhou Hagström (University of California Davis) Nelson Nientsu Hua (Paul Scherrer Institut) Oleg G. Shpyrko (University of California San Diego) Patrick Kramer (SLAC National Accelerator Laboratory) Pooja Rao (University of California Davis) Roman Mankowsky (Paul Scherrer Institut) Roopali Kukreja (University of California Davis) Sanghoon Song (SLAC National Accelerator Laboratory) Serhane Zerdane (Paul Scherrer Institut (PSI)) Shih-Wen Huang (Paul Scherrer Institut) Simon Gerber (PSI - Paul Scherrer Institut) Spencer Jeppson (University of California Davis) Surya Teja Botu (University of California Davis) Takahiro Sato (SLAC National Accelerator Laboratory) Vincent Esposito (SLAC National Accelerator Laboratory) Yanwen Sun (SLAC National Accelerator Laboratory)

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