27–30 Jun 2022
Université de Fribourg
Europe/Zurich timezone

【505】Direct determination of the electron-phonon interaction in CaTiO3 thin films

28 Jun 2022, 15:15
15m
Room G 120

Room G 120

Talk New prospects in ARPES for quantum materials New prospects in ARPES for quantum materials

Speaker

Eduardo Bonini Guedes

Description

In Fermi liquids, electron-boson coupling is (EBI) quantified through the Eliashberg function $\alpha^2F(\omega,\mathbf{k})$, which modifies their self-energy $\Sigma(\varepsilon,\mathbf{k})$ obtainable from ARPES. We present a combined ARPES, density-functional theory, and high-resolution electron energy-loss spectroscopy (HREELS) study on the EBI in CaTiO$_3$ (CTO) thin films. CTO hosts a 2-dimensional electron liquid (2DEL) analogous to that in SrTiO$_3$-based surfaces, making both materials technologically appealing for oxide electronics. Our results show that the presence of localized in-gap states changes the dielectric response of the CTO film, red-shifting high-energy phonon modes, thereby indicating their strong coupling to the 2DEL states. Combining ARPES with HREELS is a powerful approach to study quantum materials with strong EBI.

Primary author

Eduardo Bonini Guedes

Co-authors

Mr Thomas P. van Waas (UCLouvain) Mr Markus Döttling (Heisenberg Spin-dynamics Group, Physikalisches Institut, Karlsruhe Institute of Technology, Karlsruhe, Germany) Prof. Samuel Poncé (UCLouvain) Dr Marco Caputo (Elettra Sincrotrone) Nicholas Clark Plumb Nicola Marzari (EPFL) Prof. Christophe Berthod (University of Geneva) Prof. Khalil Zakeri (Karlsruhe Institue of Technology) Prof. Milan Radović (Paul Scherrer Institut) Hugo Dil (EPFL)

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