27–30 Jun 2022
Université de Fribourg
Europe/Zurich timezone

【534】Bayesian optimisation of electron-boson interaction from ARPES self-energies

28 Jun 2022, 19:00
1h 30m
Hall

Hall

Poster New prospects in ARPES for quantum materials Poster Session

Speaker

Tom van Waas (Université catholique de Louvain)

Description

Electron-boson interaction is quantified through the Eliashberg function $\alpha^2F(\omega,\mathbf{k})$, accessible through the electron self-energy $\Sigma(\varepsilon,\mathbf{k})$. In ARPES, $\Sigma(\varepsilon,\mathbf{k})$ is readily extracted from the spectral function, requiring little more than a parametric expression for the quasiparticle dispersion $\xi(\mathbf{k})$ in order to discern the photoemission kink resulting from $\Sigma(\varepsilon,\mathbf{k})$. However, $\alpha^2F(\omega,\mathbf{k})$ is highly sensitive to the parameters of $\xi(\mathbf{k})$, which itself can be difficult to determine in the presence of strong electron-boson interaction. We will describe a self-consistent and simultaneous Bayesian optimisation method for $\Sigma(\varepsilon,\mathbf{k})$ and $\xi(\mathbf{k})$, yielding the most probable $\alpha^2F(\omega,\mathbf{k})$ in an automated fashion. This optimisation allows us to discern between bosonic contributions and orbital hybridisation in ARPES spectral functions.

Authors

Eduardo Bonini Guedes Tom van Waas (Université catholique de Louvain) Hugo Dil (EPFL)

Presentation materials

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