【125】 Role of the antisymmetric exchange in quantum spin liquids

24 Aug 2017, 15:15
15m
Talk Condensed Matter Physics (incl. NESY) Condensed Matter Physics (incl. NESY)

Speaker

Mr Péter Szirmai (Laboratory of Physics of Complex Matter, Ecole Polytechnique Fédérale de Lausanne, Switzerland)

Description

Quantum spin liquids (QSL) exhibit large sensitivity to perturbations,such as the Dzyaloshinskii-Moriya (DM) interaction.Using the combination of Electron Spin Resonance (ESR) and Muon Spin Rotation ($\mu$SR),we studied the DM interaction in QSL candidates.In the triangular-lattice QSL,$\kappa$-(BEDT-TTF)$_2$Ag$_2$(CN)$_3$,our ESR measurements found a staggered moment of $\mu_{\text{s}}$=6$\times$10$^{-3}\mu_{\text{B}}$.The magnetic field dependence of the ESR-linewidth proves $\mu_{\text{s}}$ to stem from the DM interaction.In a new quasi-one-dimensional QSL,(EDT-TTF-CONH$_2$)$_2^+$BABCO$^-$,our ESR and $\mu$SR study confirmed absence of magnetic ordering down to 20mK,partially due to the highly disordered BABCO$^-$ molecular rotor layer.The ESR-linewidth and longitudinal-field $\mu$SR measurements reveal one-dimensional diffusive spin excitations.Despite the sizable DM interaction,the staggered moment remains negligible,owing to the strong disorder introduced by the anion layer.

Primary authors

Mr Péter Szirmai (Laboratory of Physics of Complex Matter, Ecole Polytechnique Fédérale de Lausanne, Switzerland) Prof. László Forró (Laboratory of Physics of Complex Matter, Ecole Polytechnique Fédérale de Lausanne, Switzerland) Dr Cécile Mézière (Laboratoire MOLTECH-Anjou, CNRS and Université d’Angers, France) Prof. Patrick Batail (Laboratoire MOLTECH-Anjou, CNRS and Université d’Angers, France) Dr Christopher Baines (Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institute, Switzerland) Stephen Cottrell (ISIS Muon Group, STFC, Great Britain) Dr Takaaki Hiramatsu (Faculty of Agriculture, Meijo University, Japan) Prof. Gunzi Saito (Faculty of Agriculture, Meijo University, Japan) Dr Bálint Náfrádi (Laboratory of Physics of Complex Matter, Ecole Polytechnique Fédérale de Lausanne, Switzerland)

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