26–30 Aug 2019
Universität Zürich
Europe/Zurich timezone

【140】Superfluorescence from lead halide perovskite quantum dot superlattices

30 Aug 2019, 13:30
15m
G 95

G 95

Talk Condensed Matter Physics (KOND) Condensed Matter Physics

Speaker

Mr Michael A. Becker (IBM Research - Zurich)

Description

Superfluorescence is a many-body collective coupling phenomenon, where coherence is established through spontaneously triggered correlations of quantum fluctuations from initially fully uncorrelated excited emitters. Here, we investigate densely packed cuboidal arrays of fully inorganic cesium lead halide perovskite quantum dots, known as superlattices and we observe key signatures of superfluorescence: A more than twenty-fold accelerated radiative decay with dynamically red-shifted emission, photon bunching, extension of the first-order coherence time and an intensity-dependent time delay after which the photon burst is emitted. Also, at high excitation density, the superfluorescent decay exhibits a Burnham-Chiao ringing behavior, reflecting the coherent Rabi-type interaction.

References:
Rainò, G.; Becker, M.A.; Bodnarchuk, M.I.; Mahrt, R.F.; Kovalenko, M.; Stöferle, T.; Nature, 563, 671-675, (2018)

Author

Mr Michael A. Becker (IBM Research - Zurich)

Co-authors

Dr Gabriele Raino (ETH Zurich) Dr Maryna I. Bodnarchuk (EMPA) Dr Rainer F. Mahrt (IBM Research - Zurich) Prof. Maksym Kovalenko (ETH Zurich) Dr Thilo Stoeferle (IBM Research - Zurich)

Presentation materials

There are no materials yet.