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5–11 Jun 2022
McMaster University
America/Toronto timezone
Welcome to the 2022 CAP Congress Program website! / Bienvenue au siteweb du programme du Congrès de l'ACP 2022!

Charge Density Wave Order and Fluctuations above T_CDW and below Superconducting T_c in the Kagome Metal CsV3Sb5

6 Jun 2022, 17:00
15m
MDCL 1010 (McMaster University)

MDCL 1010

McMaster University

Oral (Non-Student) / Orale (non-étudiant(e)) Condensed Matter and Materials Physics / Physique de la matière condensée et matériaux (DCMMP-DPMCM) M3-2 Unconventional superconductivity and topology (DCMMP) | Supraconductivité non conventionnelle et topologie (DPMCM)

Speaker

Dr Qiang Chen (Department of Physics and Astronomy, McMaster University)

Description

The phase diagram of the kagome metal family AV$_3$Sb$_5$ (A = Cs, Rb, K) features both superconductivity and charge density wave (CDW) instabilities, which have generated tremendous recent attention. Nonetheless, significant questions regarding the nature of the CDW states remain. In particular, the temperature evolution and demise of the CDW state has not been extensively studied, and little is known about the co-existence of the CDW with superconductivity at low temperatures. We report an x-ray scattering study of CsV$_3$Sb$_5$ over a broad range of temperatures from 300 K to $\sim$ 2 K, below the onset of its superconductivity at $\textit{T}_\text{c}\sim$ 2.9 K. Order parameter measurements of the $2\times2\times2$ CDW structure show an unusual and extended linear temperature dependence onsetting at $T^*$ $\sim$ 160 K, much higher than the susceptibility anomaly associated with CDW order at $\textit{T}_\text{CDW}=94$ K. This implies strong CDW fluctuations exist to $\sim2\times\textit{T}_\text{CDW}$. The CDW order parameter is observed to be constant from $T=16$ K to 2 K, implying that the CDW and superconducting order co-exist below $\textit{T}_\text{c}$, and, at ambient pressure, any possible competition between the two order parameters is manifested at temperatures well below $\textit{T}_\text{c}$, if at all. Anomalies in the temperature dependence in the lattice parameters coincide with $\textit{T}_\text{CDW}$ for $\textit{c}(T)$ and with $T^*$ for $a(T)$.

Primary author

Dr Qiang Chen (Department of Physics and Astronomy, McMaster University)

Co-authors

Bruce Gaulin (Brockhouse Institute for Materials Research, McMaster University and Department of Physics and Astronomy, McMaster University and Canadian Institute for Advanced Research) Dr Claudia Felser (Max Planck Institute for Chemical Physics of Solids, 01187 Dresden, Germany) Dr Dong Chen (Max Planck Institute for Chemical Physics of Solids, 01187 Dresden, Germany) Dr Walter Schnelle (Max Planck Institute for Chemical Physics of Solids, 01187 Dresden, Germany)

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