18–22 May 2025
Peppermill Reno
US/Pacific timezone

C1Po3C-02: Ensuring High-Purity Liquid Argon for the LBNF FDC: Collaborative Cryogenics Research Between UNICAMP and Fermilab

19 May 2025, 14:00
2h
Exhibit Hall, Tuscany Ballroom

Exhibit Hall, Tuscany Ballroom

Speaker

Roza Doubnik (Fermilab)

Description

The Long-Baseline Neutrino Facility (LBNF) located at the Sanford Underground Research Facility (SURF) in Lead, South Dakota, hosts the Deep Underground Neutrino Experiment (DUNE). This experiment employs cryostats containing nearly 70,000 metric tons of high-purity liquid argon (LAr). Ensuring LAr purity is critical for achieving the required electron lifetime, which directly impacts the experiment’s signal-to-noise ratio. The Horizontal Drift (HD) detector demands an electron lifetime exceeding 3 ms within its 3.5 m drift, equivalent to less than 100 parts-per-trillion (ppt) Oxygen contamination, while the Vertical Drift (VD) detector requires over 6 ms electron lifetime within its 6.0 m drift, corresponding to less than 50 ppt Oxygen contamination. To mitigate Nitrogen (N2) quenching of scintillation light, N2 contamination must remain below 1 ppm, as higher levels can result in up to a 20 % loss of light.
The Brazil State University of Campinas (UNICAMP) significantly contributes to LBNF FDC through the development of argon purification and regeneration systems for HD and VD cryostats.
UNICAMP designed and constructed the Purification Liquid Argon Cryostat (PuLArC), a small-scale test facility holding approximately 90 liters of LAr. Tests using PuLArC demonstrated that 1 kg of Li-FAU zeolite could reduce N₂ contamination from 20-50 ppm to 0.1-1.0 ppm within 1-2 hours. Tests at Fermilab’s Iceberg cryostat (2,625 liters) confirmed scalability, with 3 kg of Li-FAU reducing N₂ contamination from ~5 ppm to <1 ppm over 96 hours without active circulation.
This presentation will detail the research methods, test setups, and results, showcasing the potential of Li-FAU as an alternative to Molecular Sieve 4A for large-scale LAr systems. This advancement enhances DUNE's precision and demonstrates the impact of international collaboration on cryogenic research.

Author

Roza Doubnik (Fermilab)

Co-authors

Alan Hahn (Fermi National Accelerator Laboratory, PO Box 500, Batavia IL 60510, United States) Ana Amelia B. Machado (“Gleb Wataghin” Institute of Physics, UNICAMP, Campinas-SP, 13083-859, Brazil.) Cris Adriano (“Gleb Wataghin” Institute of Physics, UNICAMP, Campinas-SP, 13083-859, Brazil.) Daniel Correia (“Gleb Wataghin” Institute of Physics, UNICAMP, Campinas-SP, 13083-859, Brazil.) David Montanari (Fermi National Accelerator Laboratory, PO Box 500, Batavia IL 60510, United States) Dilson Cardoso (CPqMAE - The Research Center on Advanced Materials and Energy, Federal University of São Carlos (UFSCar), São Carlos, 13565-905, Brazil.) Dirceu Noriler (School of Chemical Engineering, UNICAMP, Campinas-SP, 13083-859, Brazil.) Elisabete M. Assaf (São Carlos Institute of Chemistry at the University of São Paulo, 13566-590, São Carlos, SP, Brazil.) Ettore Segreto (“Gleb Wataghin” Institute of Physics, UNICAMP, Campinas-SP, 13083-859, Brazil.) Flor de Maria Blaszczyk (Fermi National Accelerator Laboratory, PO Box 500, Batavia IL 60510, United States) Helio Da Motta (The Brazilian Center for Research in Physics (CBPF), Rio de Janeiro-RJ, 22290-180, Brazil.) Jose Mansur Assaf (CPqMAE - The Research Center on Advanced Materials and Energy, Federal University of São Carlos (UFSCar), São Carlos, 13565-905, Brazil.) Magda B. Fontes (The Brazilian Center for Research in Physics (CBPF), Rio de Janeiro-RJ, 22290-180, Brazil.) Mark Adamowski (Fermi National Accelerator Laboratory, PO Box 500, Batavia IL 60510, United States) Pascoal José Giglio Pagliuso (“Gleb Wataghin” Institute of Physics, UNICAMP, Campinas-SP, 13083-859, Brazil.) Robert Mrowca (Fermi National Accelerator Laboratory, PO Box 500, Batavia IL 60510, United States) Rosembergue G. Gonçalves (CPqMAE - The Research Center on Advanced Materials and Energy, Federal University of São Carlos (UFSCar), São Carlos, 13565-905, Brazil.) Thiago P.M. Alegre (“Gleb Wataghin” Institute of Physics, UNICAMP, Campinas-SP, 13083-859, Brazil.) Zack West (Fermi National Accelerator Laboratory, PO Box 500, Batavia IL 60510, United States)

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