28–31 Aug 2018
EPFL
Europe/Zurich timezone

【914】 Single-Shot Broadband Femtosecond Circular Dichroism in the Deep-UV

29 Aug 2018, 17:45
15m
CE 5 (EPFL)

CE 5

EPFL

Talk Biophysics, Medical Physics and Soft Matter Biophysics, Medical Physics and Soft Matter

Speaker

Dr Malte Oppermann (Laboratory of Ultrafast Spectroscopy, EPFL)

Description

Circular dichroism (CD) spectroscopy is a well-established tool in analytical biochemistry. In the deep-UV range (< 300 nm), it is sensitive to the spatial arrangement of transition dipoles on amino acid residues, nucleotides and peptides. Time-resolved CD spectroscopy is thus a promising experimental technique that is sensitive to changes in biomolecular configuration as a function of time, combining the time-dependent electronic information provided by traditional transient absorption spectroscopy with the structural information encoded in the chirality of molecular systems. In this context, we now report the first single-shot broadband circular dichroism spectrometer in the deep-UV (250–370 nm) with femtosecond time-resolution. Artefact-free static and transient CD spectra of enantiopure [Ru(bpy)$_3$]$^{2+}$ are successfully recorded at noise levels < 10$^{-5}$ OD.

Authors

Dr Malte Oppermann (Laboratory of Ultrafast Spectroscopy, EPFL) Mr Benjamin Bauer Mr Thomas Rossi Dr Frank van Mourik Prof. Majed Chergui

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